CuO/LaCoO3催化合成气制C2 醇反应性能研究任务书

 2021-10-23 21:46:28

1. 毕业设计(论文)的内容和要求

1. 查阅、整理文献资料,加深对自己课题的理解,并撰写开题报告。

2. 要求学生对化工原理、无机与分析化学、仪器分析等学科复习,从而对以后催化剂性能测试实验、表征分析打下基础。

3. 主要研究采用柠檬酸络合法制备LaCoO3钙钛矿型复合氧化物,并用等体积浸渍法将相应的铜元素负载到钙钛矿结构上。

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2. 参考文献

[1]. 阚泉生. 合成气合成低碳醇催化剂的制备与工艺研究[D].西安工程大学,2015.[2]. Mingyue Ding,Minghuang Qiu,Jianguo Liu,Yuping Li,Tiejun Wang,Longlong Ma,Chuangzhi Wu. Influence of manganese promoter on co-precipitated FeCu based catalysts for higher alcohols synthesis[J]. Fuel,2013,109.[3]. Minggui Lin,Kegong Fang,Debao Li,Yuhan Sun. CO hydrogenation to mixed alcohols over co-precipitated CuFe catalysts[J]. Catalysis Communications,2008,9(9).[4]. Ruili, Lu, Dongsen, et al. Enhanced activity of CuFe/SiO2 catalyst for CO hydrogenation to higher alcohols by pretreating the support with ammonia[J]. Journal of Industrial Engineering Chemistry, 2015.[5]. Yang Q , Liu G , Liu Y . Perovskite-type Oxides as the Catalyst Precursors for Preparing Supported Metallic Nanocatalysts: A Review[J]. Industrial Engineering Chemistry Research, 2017:acs.iecr.7b03251.[6]. Xiang Y , Barbosa R , Kruse N . Higher Alcohols through CO Hydrogenation over CoCu Catalysts: Influence of Precursor Activation[J]. Acs Catalysis, 2014, 4(8):2792-2800.[7]. Nguyen Tien-Thao,M. Hassan Zahedi-Niaki,Houshang Alamdari,Serge Kaliaguine. Effect of alkali additives over nanocrystalline CoCu-based perovskites as catalysts for higher-alcohol synthesis[J]. Journal of Catalysis,2006,245(2).[8]. Guiping Jiao, Yunjie Ding, Hejun Zhu,等. Effect of La2O3 doping on syntheses of C1C18 mixed linear α-alcohols from syngas over the Co/AC catalysts[J]. applied catalysis a general, 2009, 364(1-2):137-142.[9]. Wang Z , Spivey J J . Effect of ZrO2, Al2O3 and La2O3 on cobalt-copper catalysts for higher alcohols synthesis[J]. Applied Catalysis A General, 2015, 507:S0926860X15301654.[10]. H. He,H.X. Dai,L.H. Ng,K.W. Wong,C.T. Au. Pd-, Pt-, and Rh-Loaded Ce 0.6 Zr 0.35 Y 0.05 O 2 Three-Way Catalysts: An Investigation on Performance and Redox Properties[J]. Journal of Catalysis,2002,206(1).[11]. Hideaki Muraki,Geng Zhang. Design of advanced automotive exhaust catalysts[J]. Catalysis Today,2000,63(2).[12]. Voorhoeve, RHJ, Remeika, JP, FREELAND, PE,等. Rare-Earth Oxides of Manganese and Cobalt Rival Platinum for the Treatment of Carbon Monoxide in Auto Exhast[J]. Science, 1972, 177(4046):353-354.[13]. Ocal M , Oukaci R , Marcelin G , et al. Steady State Isotopic Transient Kinetic Analysis (SSITKA) Investigation of NO Reduction with CO over Perovskite Catalysts[J]. Industrial Engineering Chemistry Research, 1994, 33(12):2930-2934.[14]. Lindstedt A , Str?Mberg D , Milh M A . High-temperature catalytic reduction of nitrogen monoxide by carbon monoxide and hydrogen over La1?xSrxMO3 perovskites (M = Fe, Co) during reducing and oxidising conditions[J]. 1994, 116(1-2):109-126.[15]. Yu.I. Pyatnitsky,N.I. Ilchenko,L.Yu. Dolgikh,N.V. Pavlenko. Methane oxidative coupling over SrCoO 3 -based perovskites in periodic regime[J]. Topics in Catalysis,2000,11-12(1-4).[16]. Parvulescu V I , Grange P , Delmon B . Catalytic removal of NO[J]. 1998, 46(4):233-316.[17]. Giebeler L , Kiessling D , Wendt G . LaMnO3 Perovskite Supported Noble Metal Catalysts for the Total Oxidation of Methane[J]. Chemical Engineering Technology, 2007, 30(7):889-894.[18]. 韩通. 钙钛矿为前驱体的负载型铑基催化剂用于合成气制备低碳醇反应的研究[D].天津大学,2016.

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