1. 毕业设计(论文)的内容和要求
本课题将设计合成铁氮双掺杂多孔碳材料,用以电化学检测H2O2。
通过优化合成条件,来制备高比表面积、多活性位点的多孔碳材料,实现高效快速检测双氧水的目的。
在这一基础上,通过表征、分析催化剂的结构,研究实验条件对催化剂组成的影响、以及与催化性能的关系。
2. 参考文献
毕设期间要进行研究现状调查与总结,要求在开题报告及毕业设计(论文)中涉及的英文文献不少于20篇,其中近5年不少于8篇,英文文献不少于5篇。
以下是与本课题相关的部分文献列表:[1]徐朝权.铁氮共掺杂多孔碳材料的制备及其氧还原性能研究[D].新疆:新疆大学,2018.[2]张璐.铁氮共掺杂的多孔碳材料MFC阴极的制备与催化性能研究[D].黑龙江哈尔滨:哈尔滨工业大学,2018.[3]贺新福,龙雪颖,吴红菊,等.氮掺杂石墨烯/多孔碳复合材料的制备及其氧还原催化性能[J].化工学报,2019,70(6):2308-2315.[4]吴雪艳,王开学,陈接胜,多孔碳材料的制备[J].化学进展,2012,24(2/3):262-274.[5]余正发,王旭珍,刘宁,等.N掺杂多孔碳材料研究进展[J].化工进展,2013,32(4):824-862.[6]袁雪,丁硕,徐大为,刘雪美,张美茜,刘建华,戴昉纳.NP共掺杂的多孔碳材料在氧还原方面的应用.[J].聊城大学学报,2019,32(2):80-84.[7]宋开绪,崔丽莉,何兴权.铁氮共掺多孔碳材料的制备及其ORR性能研究[J].长春理工大学学报,2019,42(3):96-101.[8]杨慧聪,梁骥,王振兴,等.多孔碳质材料在氧还原电催化中的应用[J].新型炭材,2016,3:243-263[9]杨文秀,郏建波.铁掺杂的多孔碳复合材料的制备及其氧还原研究[C].∥中国化学会第29届学术年会摘要集第4分会:纳米生物传感新方法,2014.[10]Wang L,Shen H,Gao S,et al.Atomically Dispersed Fe,N Co-Doped Ordered Mesoporous Carbon for Non-Enzymatic Hydrogen Peroxide Sensing[J].Journal of The Electrochemical Society,2018,165(7):H348-H352.[11]Dhara K,Mahapatra D R.Recent advances in electrochemical nonenzymatic hydrogen peroxide sensors based on nanomaterials:a review[J].Journal of Materials Science,1-39.[12]Wang Z,Dai Z.Carbon nanomaterial-based electrochemical biosensors:an overview[J].Nanoscale,2015,7(15):6420-6431.[13]Chen S,Yuan R,Chai Y,et al.Electrochemical sensing of hydrogen peroxide using metal nanoparticles:a review[J].Microchimica Acta,2013,180(1-2):15-32.[14]Nakabayashi Y,Yoshikawa H.Amperometric biosensors for sensing of hydrogen peroxide based on electron transfer between horseradish peroxidase and ferrocene as a mediator[J].Analytical Sciences,2000,16(6):609-613.[15]Patella B,Inguanta R,Piazza S,et al.A nanostructured sensor of hydrogen peroxide[J].Sensors and Actuators B:Chemical,2017,245:44-54.[16]Wang M,Jiang X,Liu J,et al.Highly sensitive H2O2 sensor based on Co3O4 hollow sphere prepared via a template-free method[J].Electrochimica Acta,2015,182:613-620.[17]Santhosh C,Deivasegamani R,Nivetha R,et al.A non-enzymatic sensor for hydrogen peroxide based on the use of α-Fe2O3 nanoparticles deposited on the surface of NiO nanosheets[J].Microchimica Acta,2017,184(9):3223-3229.[18]Cao G S,Wang P,Li X,et al.A sensitive nonenzymatic hydrogen peroxide sensor based on Fe3O4Fe2O3 nanocomposites[J].Bulletin of Materials Science,2015,38(1):163-167.[19]Majumder S,Saha B,Dey S,et al.A highly sensitive non-enzymatic hydrogen peroxide and hydrazine electrochemical sensor based on 3D micro-snowflake architectures of α-Fe2O3[J].RSC Advances,2016,6(65):59907-59918.[20]Cai J,Ding S,Chen G,et al.In situ electrodeposition of mesoporous aligned α-Fe2O3 nanoflakes for highly sensitive nonenzymatic H2O2 sensor[J].Applied Surface Science,2018,456:302-306.
